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    Arsenic and trace metal concentrations in different vegetable types and assessment of health risks from their consumption
    (Elsevier, 2022) Varol, Memet; Gündüz, Kazım; Sünbül, Muhammet Raşit; Aytop, Halil
    The levels of 12 trace metal (loid)s (TMs) in 10 vegetable types including leafy vegetables (purslane, purple basil and parsley) and fruiting vegetables (pepper, tomato, eggplant, cucumber, zucchini, green bean and melon) and in maize grown in Malatya province (Turkey) were investigated and non-carcinogenic health risks from consumption of these crops were assessed. The levels of TMs were measured by inductively coupled plasma-optical emission spectrometry. The mean levels of Ni, Cu, Cd, Cr, As and Zn in all crops were below maximum permissible concentrations (MPCs), while those of Pb in pepper (0.109 mg/kg fw), eggplant (0.103 mg/kg fw) and green bean (0.177 mg/kg fw) slightly exceeded MPCs (0.1 mg/kg fw). Leafy vegetables had relatively higher concentrations of Al, As, Ba, Cr, Cu, Fe and Mn compared to fruiting vegetables and maize. The estimated daily intake value of each TM estimated for each crop was found to be below the tolerable daily intake value. The target hazard quotients of all TMs in all crops did not exceed the acceptable non-carcinogenic risk level. However, hazard index (HI) value (1.57) in tomato was found to be above the threshold value of 1, indicating non-carcinogenic risks for consumers due to the intake of combined TMs in tomato. The THQ values of As, Co and Pb contributed 46.4%, 24.5% and 16.4% of the HI value of tomato, respectively. High daily consumption amount of tomato likely resulted in high HI value. The findings obtained in this study reveal that even if the levels of TMs in vegetables are safe, more attention should be paid to non-carcinogenic risks associated with TMs as a result of high vegetable intake.
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    Environmental, ecological and health risks of trace elements, and their sources in soils of Harran Plain, Turkey
    (Elsevier, 2020) Varol, Memet; Sünbül, Muhammet Raşit; Aytop, Halil; Yılmaz, Cafer Hakan
    Soil pollution with trace elements (TEs) has become an increasingly serious environmental concern, however, assessment of ecological and human health risks especially in intensive agricultural regions remains limited. In this study, the contents of ten TEs (Al, As, Pb, Cr, Cu, Zn, Ni, Co, Mn and Fe) in soil samples from 204 sampling sites in the Harran Plain (Turkey) were examined to evaluate possible sources, pollution status and environmental, ecological and health risks of these elements. Only As and Ni exceeded the upper continental crust concentrations. Among ten TEs, Ni and As had the highest mean values of enrichment factor (EF) and contamination factor (Cf), indicating that soils showed moderate enrichment and moderate contamination with these elements. Ecological risk factor and ecological risk index values of all samples were <40 and <150, respectively, indicating low ecological risk in the study area. Factor analysis and correlation analysis indicated that Al, Pb, Cr, Cu, Zn, Co, Mn and Fe mainly originated from natural sources, Ni from mixed sources of anthropogenic and lithogenic origins, while arsenic primarily originated from anthropogenic activities. The hazard quotient values for both adults and children did not exceed 1, suggesting that all TEs in soil through ingestion, dermal contact and inhalation pathways had no significant non-carcinogenic risks. Children were more susceptible to non-carcinogenic health effects of TEs in soils. The carcinogenic risk values of As, Co, Cr and Ni were within the acceptable risk range, indicating that carcinogenic risks were not expected.